UPDATED FORMULA:
You can achieve this by using the "Items" property of the ComboBox and the "Concatenate" and Split function to concatenate the text from all the labels.
Here's an example formula that you can use for the "Items" property of the ComboBox:
Split(Concatenate(Label4_1.Text, ",", Label4_2.Text, ",", Label4_3.Text, ",", Label4_4.Text, ",", Label4_5.Text, ",", Label4_6.Text, ",", Label4_7.Text, ",", Label4_8.Text, ",", Label4_9.Text, ",", Label4_10.Text, ",", Label4_11.Text, ",", Label4_12.Text, ",", Label4_13.Text, ",", Label4_14.Text, ",", Label4_15.Text, ",", Label4_16.Text, ",", Label4_17.Text, ",", Label4_18.Text, ",", Label4_19.Text, ",", Label4_20.Text), ",")
This formula concatenates the text from all the labels using commas as separators, then splits resulting string by the comma as the items for the ComboBox.
Note that if you add or remove labels, you'll need to adjust the formula accordingly.
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Rick Hurt